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The chances for B.Tech CSE are moderate, but chances for ECE and EE are high.

You have not written about the total marks of PCM out of which he scored 135 marks. However if the total marks for PCM are 300, than percentage of marks obtained by your brother is 45%. Which is not enough for getting admission in Engineering colleges. The minimum marks required in PCM are about 50% for major engineering admissions.

You have not written about the home state you belongs. However on the basis of your JEE Main rank, The following are the best colleges under other state quota.
1. MNNIT Allahabad
2. NIT Warangal
3. MNIT Jaipur
4. NIT Surathkal
5. NIT Bhopal.

Currently as per now I would suggest B.Tech CSE as its covering all possible emerging technologies required in corporate and IT industry but if your interested AI and Ml then you can opt for specialisation in the B.Tech CSE AI ML which mainly focus Practical learning of Machine learning and artificial intelligence which will help you to make your career in that field apart from being just B.Tech CSE engineering based careers.

Yes, you will get NIT Jamshedpur But I think you are not able to get your desired Branch. I suggest irrespective of the College you should go for the NIT's in which you get your desired or better Branch. But if you want NIT Jamshedpur irrespective of Branch then Might be you will get till last round of counselling. One more suggestion In counselling go till last Round, You might be getting a good branch with better college.

Candidates shall appear for KSET in their relevant subject of their post-graduation only, in case the candidate did not find the subject of his/her post-graduation in the list of KSET subjects, the candidate may appear in UGC NET / UGC-CSIR NET which is held twice a year.

Yes, offcourse you can do MBA from London if you are eligible for the criteria of London University.